Title: Unified Crystal-field Picture for Actinide Dioxides
Authors: MAGNANI NicolaAMORETTI G.CARRETTA S.SANTINI P.CACIUFFO ROBERTO
Citation: JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS vol. 68 no. 11 p. 2020-2023
Publisher: PERGAMON-ELSEVIER SCIENCE LTD
Publication Year: 2007
JRC Publication N°: JRC42502
ISSN: 0022-3697
URI: http://dx.doi.org/10.1016/j.jpcs.2007.08.052
http://publications.jrc.ec.europa.eu/repository/handle/JRC42502
DOI: 10.1016/j.jpcs.2007.08.052
Type: Articles in Journals
Abstract: We present a perturbative model for crystal-field calculations in f-electron compounds, which keeps into account the mixing between states labelled by different total angular momentum J. We use this model to analyze the results of inelastic neutron scattering experiments on actinide dioxides accumulated over a number of years. By comparing our calculations with the published results of other experiments, we point out that a unified crystal-field picture for this series of compounds clearly emerges.
JRC Institute:Institute for Transuranium Elements

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