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Anomalies in the Charge Yields of Fission Fragments from the 238U(n,f) Reaction

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Fast-neutron-induced fission of 238U at an energy just above the fission threshold is studied with a novel technique which involves the coupling of a high-efficiency γ-ray spectrometer (MINIBALL) to an inverse-kinematics neutron source (LICORNE) to extract charge yields of fission fragments via γ−γ coincidence spectroscopy. Experimental data and fission models are compared and found to be in reasonable agreement for many nuclei; however, significant discrepancies of up to 600% are observed, particularly for isotopes of Sn and Mo. This indicates that these models significantly overestimate the standard 1 fission mode and suggests that spherical shell effects in the nascent fission fragments are less important for low-energy fast-neutron-induced fission than for thermal neutron-induced fission. This has consequences for understanding and modeling the fission process, for experimental nuclear structure studies of the most neutron-rich nuclei, for future energy applications (e.g., Generation IV reactors which use fast-neutron spectra), and for the reactor antineutrino anomaly.
2017-08-01
AMER PHYSICAL SOC
JRC105932
0031-9007,   
https://journals.aps.org/prl/abstract/10.1103/PhysRevLett.118.222501,    https://publications.jrc.ec.europa.eu/repository/handle/JRC105932,   
10.1103/PhysRevLett.118.222501,   
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