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|Title:||Tricritical point from high-field magnetoelastic and metamagnetic effects in UN|
|Authors:||SHRESTHA K; ANTONIO D.; JAIME MARCELO; HARRISON N.; MAST DANIEL; SAFARIK D.; DURAKIEWICZ T.; GRIVEAU JEAN-CHRISTOPHE; GOFRYK KRZYSZTOF|
|Citation:||SCIENTIFIC REPORTS vol. 7 p. 6642|
|Publisher:||NATURE PUBLISHING GROUP|
|Type:||Articles in periodicals and books|
|Abstract:||Uranium nitride (UN) is one of the most studied actinide materials as it is a promising fuel for the next generation of nuclear reactors. Despite large experimental and theoretical efforts, some of the fundamental questions such as degree of 5 f–electron localization/delocalization and its relationship to magneto-vibrational properties are not resolved yet. Here we show that the magnetostriction of UN measured in pulsed magnetic fields up to 65 T and below the Néel temperature is large and exhibits complex behavior with two transitions. While the high field anomaly is a field-induced metamagnetic-like transition and affects both magnetisation and magnetostriction, the low field anomaly does not contribute to the magnetic susceptibility. Our data suggest a change in the nature of the metamagnetic transition from first to second order-like at a tricritical point at T tri ∼ 24 K and H tri ∼ 52 T. The induced magnetic moment at 60 T might suggest that only one subset of magnetic moments has aligned along the field direction. Using the results obtained here we have constructed a magnetic phase diagram of UN. These studies demonstrate that dilatometry in high fields is an effective method to investigate the magneto-structural coupling in actinide materials.|
|JRC Directorate:||Nuclear Safety and Security|
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