Classification of uranium ore concentrates applying support vector machine to spectrophotometric and textural features

Uranium ore concentrates (UOCs) are produced in the early stages of the nuclear fuel cycle, prior to conversion to uranium hexafluoride. Because of their high uranium content and the large-scale production, UOCs diversion from civilian use and proliferation are potential risks. This implies the necessity to develop methods able to recognize characteristic parameters correlating each UOC powder to its history and origin. Here, a novel methodology is proposed: first the reflectance spectra of 79 commercial UOCs are acquired and clustered by means of Ward’s clustering analysis, then classified by Support Vector Machine (SVM). Second, SVM classification is applied to the image textural features extracted with the Grey Level Cooccurrence Matrix (GLCM) and the Angle Measure Technique (AMT) algorithms for powders in two different colour groups. The developed SVM models present good classification quality: a Matthews correlation coefficient (MCC) of 0.95 is obtained for the classification based on colours while macro-F1 is generally greater than 0.81 (MCC larger than 0.75) for the texture-based classification. These results reveal the potentiality of the present automated classification for the scopes of nuclear forensics in the identification of an unknown uranium ore concentrate sample.

MARCHETTI Mara;  FONGARO Lorenzo;  BULGHERONI Antonio;  WALLENIUS Maria;  MAYER Klaus; 

2022-09-22

PERGAMON-ELSEVIER SCIENCE LTD

JRC128413

0883-2927 (online),   

https://www.sciencedirect.com/science/article/pii/S0883292722002475,    https://publications.jrc.ec.europa.eu/repository/handle/JRC128413,   

10.1016/j.apgeochem.2022.105443 (online),