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|Title:||Characterization of the 222-Rn Family Turbulent Transport in the Convective Atmospheric Boundary Layer|
|Authors:||VINUESA JEAN; GALMARINI STEFANO|
|Citation:||ATMOS. CHEM. PHYS. (DISCUSS.) vol. 6 no. 5 p. 8917-8960|
|Publisher:||EUROPEAN GEOSCIENCES UNION|
|Type:||Articles in periodicals and books|
|Abstract:||The combined effect of turbulent transport and radioactive decay on the distribution of 222-Rn and its progeny in convective atmospheric boundary layers (CBL) are investigated. Large eddy simulation is used to simulate their dispersion in steady state CBL and in unsteady conditions represented by the growth of a CBL within a pre-existing reservoir layer. The exact decomposition of the concentration and flux budget equations under steady state conditions allowed us to determine which processes are responsible for the vertical distribution of 222-Rn and its progeny. Their mean concentrations are directly correlated with their half-life, e.g. 222-Rn and 210-Pb are the most abundant whereas 218-Po show the lowest concentrations. 222-Rn flux decreases linearly with height and its flux budget is similar to the one of inert emitted scalar, i.e., a balance between on the one hand the gradient and the buoyancy production terms, and on the other hand the pressure and dissipation at smaller scales which tends to destroy the fluxes. While 222-Rn exhibits the typical bottom-up behavior, the maximum flux location of the daughters is moving upwards while their rank in the 222-Rn progeny is increasing leading to a typical top-down behavior for 210-Pb. We also found that 222-Rn short-lived daughters, e.g. 218-Po and 214-Pb, have relevant radioactive decaying contributions acting as flux sources leading to deviations from the linear flux shape. In addition, while analyzing the vertical distribution of the radioactive decay contributions to the concentrations, i.e. the decaying zone, we found a discrepancy in height of 222-Rn daughters' radioactive transformations. Under unsteady conditions, the same behaviors reported under steady state conditions are found: deviation of the fluxes from the linear shape for 218-Po, enhanced discrepancy in height of the radioactive transformation contributions for all the daughters. In addition, 222-Rn and its progeny concentrations collapse due to the rapid growth of the CBL. The analysis emphasizes the crucial role of turbulent transport in the behavior of 222-Rn morning concentrations, in particular the ventilation at the top of the boundary layer that leads to the dilution of 222-Rn by mixing with radon low concentration air.|
|JRC Directorate:||Sustainable Resources|
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