Nature of Non-magnetic Strongly-correlated State in d-Plutonium
Ab initio relativistic dynamical mean-field theory is applied to resolve the longstanding
controversy between theory and experiment in the simple; face-centered cubic phase
of plutonium. In agreement with experiment, neither static nor dynamical magnetic moments are predicted. In addition, the quasiparticle density of states reproduces not only the peak close to the Fermi level, which explains the large coefficient of electronic specific heat, but also main 5f features observed in photoelectron spectroscopy.
POUROVSKII L.V.;
KATSNELSON M.I.;
LICHTENSTEIN A.I.;
HAVELA Ladislav;
GOUDER Thomas;
WASTIN Franck;
SHICK A.B.;
DRCHAL V.;
LANDER Gerard;
2006-08-16
E D P SCIENCES
JRC34404
https://publications.jrc.ec.europa.eu/repository/handle/JRC34404,
10.1209/epl/i2005-10548-5,
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