We characterized, for the first time, submicro- and nanosized fission product-alloy particles that were extracted nondestructively from spent nuclear fuel, in terms of noble metal (Mo–Ru–Tc–Rh–Pd–Te) composition, atomic level homogeneity and lattice parameters. The evidences obtained in this work contribute to an improved understanding of the redox chemistry of radionuclides in nuclear waste repository environments and, in particular, of the catalytic properties of these unique metal alloy particles.
CUI Daqing;
RONDINELLA Vincenzo;
FORTNER J. A.;
KROPF A. J.;
ERIKSSON L.;
WRONKIEWICZ D.J.;
SPAHIU K.;
2012-12-14
ELSEVIER SCIENCE BV
JRC75298
0022-3115,
https://publications.jrc.ec.europa.eu/repository/handle/JRC75298,
10.1016/j.jnucmat.2011.10.015,
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